resumo
The rapid miniaturization of electronic devices has pushed the limits of conventional silicon-based technologies, creating a pressing need for novel approaches to sustain the exponential growth of computing power. This study explores the innovative application of Ln3+-doped glasses in developing molecular logic systems as a potential solution. Exploiting Eu3+ and Dy3+, we investigated the luminescence properties under various physical stimuli such as excitation wavelength and temperature. Our findings reveal the capability to construct logic elements of varying complexity, from simple AND and OR gates to advanced FULL-ADDER and FULL-SUBTRACTOR circuits. This work represents the first instance of using Ln3+ exclusively for molecular logic via physical stimuli. The robust and stable optical properties of the doped glasses enable their integration into conventional electronic and photonic devices, potentially revolutionizing the landscape of molecular logic and computing. This research not only enhances the understanding of light-matter interactions in Ln3+-doped systems but also opens new pathways for the development of miniaturized, high-performance innovative computational devices.
palavras-chave
NIOBIUM
categoria
Optics
autores
Salgueiro, RF; Maturi, FE; da Silva, VMP; Manzani, D; Brites, CDS
nossos autores
Projectos
CICECO - Aveiro Institute of Materials (UIDB/50011/2020)
CICECO - Aveiro Institute of Materials (UIDP/50011/2020)
Associated Laboratory CICECO-Aveiro Institute of Materials (LA/P/0006/2020)
agradecimentos
This work was partially developed within the scope of the project CICECO-Aveiro Institute of Materials, UIDB/50011/2020 (DOI 10.54499/UIDB/50011/2020) , UIDP/50011/2020 (DOI 10.54499/UIDP/50011/2020) & LA/P/0006/2020 (DOI 10.54499/LA/P/0006/2020) , financed by national funds through the FCT/MCTES (PIDDAC) . This work was also financially supported by the LogicALL project (PTDC/CTM-CTM/0298/2020) through Portuguese funds. R.F.S. and F. E.M. acknowledge the financial support from the FCT through research grants (PTDC/CTM-CTM/0340/2021) and UI/BD/151445/2021 (DOI 10.54499/UI/BD/151445/2021) , respectively. F.E.M. acknowledges the funding received from the European Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement No. 823941 (FUNGLASS)

